Scientists find evidence of exotic state of matter in candidate material
for quantum computers

Date:
October 5, 2020
Source:
Florida State University
Summary:
Using a novel technique, scientists have found evidence for a
quantum spin liquid, a state of matter that is promising as a
building block for the quantum computers of tomorrow.



FULL STORY ========================================================================== Using a novel technique, scientists working at the Florida State
University- headquartered National High Magnetic Field Laboratory have
found evidence for a quantum spin liquid, a state of matter that is
promising as a building block for the quantum computers of tomorrow.


========================================================================== Researchers discovered the exciting behavior while studying the so-called electron spins in the compound ruthenium trichloride. Their findings,
published today in the journal Nature Physics , show that electron
spins interact across the material, effectively lowering the overall
energy. This type of behavior - - consistent with a quantum spin liquid --
was detected in ruthenium trichloride at high temperatures and in high
magnetic fields.

Spin liquids, first theorized in 1973, remain something of a
mystery. Despite some materials showing promising signs for this state
of matter, it is extremely challenging to definitively confirm its
existence. However, there is great interest in them because scientists
believe they could be used for the design of smarter materials in a
variety of applications, such as quantum computing.

This study provides strong support that ruthenium trichloride is a spin
liquid, said physicist Kim Modic, a former graduate student who worked
at the MagLab's pulsed field facility and is now an assistant professor
at the Institute of Science and Technology Austria.

"I think this paper provides a fresh perspective on ruthenium trichloride
and demonstrates a new way to look for signatures of spin liquids,"
said Modic, the paper's lead author.

For decades, physicists have extensively studied the charge of an
electron, which carries electricity, paving the way for advances
in electronics, energy and other areas. But electrons also have a
property called spin. Scientists want to also leverage the spin aspect
of electrons for technology, but the universal behavior of spins is not
yet fully understood.



==========================================================================
In simple terms, electrons can be thought of as spinning on an axis,
like a top, oriented in some direction. In magnetic materials, these spins align with one another, either in the same or opposite directions. Called magnetic ordering, this behavior can be induced or suppressed by
temperature or magnetic field. Once the magnetic order is suppressed,
more exotic states of matter could emerge, such as quantum spin liquids.

In the search for a spin liquid, the research team homed in on ruthenium trichloride. Its honeycomb-like structure, featuring a spin at each site,
is like a magnetic version of graphene -- another hot topic in condensed
matter physics.

"Ruthenium is much heavier than carbon, which results in strong
interactions among the spins," said MagLab physicist Arkady Shekhter,
a co-author on the paper.

The team expected those interactions would enhance magnetic frustration
in the material. That's a kind of "three's company" scenario in which
two spins pair up, leaving the third in a magnetic limbo, which thwarts magnetic ordering.

That frustration, the team hypothesized, could lead to a spin liquid
state.

Their data ended up confirming their suspicions.

"It seems like, at low temperatures and under an applied magnetic field, ruthenium trichloride shows signs of the behavior that we're looking for," Modic said. "The spins don't simply orient themselves depending on the alignment of neighboring spins, but rather are dynamic -- like swirling
water molecules -- while maintaining some correlation between them."
The findings were enabled by a new technique that the team developed
called resonant torsion magnetometry, which precisely measures the
behavior of electron spins in high magnetic fields and could lead to
many other new insights about magnetic materials, Modic said.



==========================================================================
"We don't really have the workhorse techniques or the analytical
machinery for studying the excitations of electron spins, like we do
for charge systems," Modic said. "The methods that do exist typically
require large sample sizes, which may not be available. Our technique
is highly sensitive and works on tiny, delicate samples. This could be a game-changer for this area of research." Modic developed the technique
as a postdoctoral researcher and then worked with MagLab physicists
Shekhter and Ross McDonald, another co-author on the paper, to measure ruthenium trichloride in high magnetic fields.

Their technique involved mounting ruthenium trichloride samples onto
a cantilever the size of a strand of hair. They repurposed a quartz
tuning fork - - similar to that in a quartz crystal watch -- to vibrate
the cantilever in a magnetic field. Instead of using it to tell time
precisely, they measured the frequency of vibration to study the
interaction between the spins in ruthenium trichloride and the applied
magnetic field. They performed their measurements in two powerful magnets
at the National MagLab.

"The beauty of our approach is that it's a relatively simple setup, which allowed us to carry out our measurements in both a 35-tesla resistive
magnet and a 65-tesla pulsed field magnet," Modic said.

The next step in the research will be to study this system in the MagLab's world-record 100-tesla pulsed magnet.

"That high of a magnetic field should allow us to directly observe the suppression of the spin liquid state, which will help us learn even more
about this compound's inner workings," Shekhter said.


========================================================================== Story Source: Materials provided by Florida_State_University. Original
written by Kristen Coyne. Note: Content may be edited for style and
length.


========================================================================== Journal Reference:
1. K. A. Modic, Ross D. McDonald, J. P. C. Ruff, Maja D. Bachmann,
You Lai,
Johanna C. Palmstrom, David Graf, Mun K. Chan, F. F. Balakirev,
J. B.

Betts, G. S. Boebinger, Marcus Schmidt, Michael J. Lawler,
D. A. Sokolov, Philip J. W. Moll, B. J. Ramshaw, Arkady
Shekhter. Scale-invariant magnetic anisotropy in RuCl3
at high magnetic fields. Nature Physics, 2020; DOI:
10.1038/s41567-020-1028-0 ==========================================================================

Link to news story: https://www.sciencedaily.com/releases/2020/10/201005170841.htm

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